FoodNet

Experimental cookery

1932

Page 449

Presented as published in 1932. Historical recipes may not meet modern food-safety standards. Cook from the modern interpretation, not the original instructions.
The hydrocarbon chain of oleic acid is not a saturated one. It contains a double bond. With a limited amount of oil on the surface of the water the double bond as well as the carboxyl group may be drawn down onto the surface of the water. In this way it covers a larger surface area of the water. Unsaturated fatty acids cover a larger surface area than satu- rated ones. Langmuir has measured the length of the molecules and the area of the water covered by them. He reports that the area covered by the three saturated acids, palmitic, stearic, and creotic, is practically the same, yet the number of carbons in palmitic is 16 and in creotic 26, the latter having the longer molecule. The glyceride tristearin covers an area three times that of one molecule of stearic acid. From this it is seen that the area, covered is the same whether as an acid or as an ester of a glyceride. In measuring the height above the surface of the water he found it to be the same as the length of the hydrocarbon chains, showing that they are packed vertically side by side. The results are probably best told in his 564 FATS AND OILS words. "The unsaturated fatty acids all cover much greater areas per molecule than the saturated. The double bond in oleic acid is thus appar- ently drawn down onto the water surface. It is interesting to note, however, that linoleic acid with its two double bonds, does not cover any greater area per molecule than oleic acid. It may be that the double bonds attract one another to some extent in place of the water. Linolenic acid, however, with three double bonds, covers a considerably greater area than oleic or linoleic. As the number of double bonds increases, the energy consumed in compressing the film decreases, probably because the carboxyl groups tend to be attracted by the double bonds in adjacent molecules and are thus more easily separated from the water surface." Polar groups of molecules and water are attracted to each other. Harkins and co-workers have reported that, if an organic liquid contains polar groups in its molecules, these groups turn towards the water, and the amount of work required to separate it from the surface of the water is greater than when the polar groups are absent. These polar groups are substances containing oxygen, nitrogen, sulfur, iodine, bromine, chlorine, or double or triple bonds. In a later paper Harkins and Cheng have reported that a paraffin with a triple bond increases the adhesional work very decidedly; they state: ''This and other studies in this paper should prove of value in study of lubrication and other adhesional phenomena." Wilson and Barnard have reported that a good lubricant is one that has the property of "oiliness." They define oiliness as "The property by virtue of which one fluid gives lower coefficients of friction (generally at slow speeds or high loads) than another fluid of the same viscosity."